In this experimental and modeling investigation, Wyodak coal, a subbituminous coal from the Powder River Basin, was the coal employed and corn stover was the biomass. Torrefied corn stover was ...
DOI: / Corpus ID: ; CO2 gasification of Powder River Basin coal catalyzed by a costeffective and environmentally friendly iron catalyst article{Zhang2015CO2GO, title={CO2 gasification of Powder River Basin coal catalyzed by a costeffective and environmentally friendly iron catalyst}, author={Fan Zhang and Deping Xu and Yonggang Wang and Morris D. Argyle ...
Introduction. Catalytic coal gasification has been studied worldwide for nearly 20 years due to its advantages, such accelerating process rate, improving carbon conversion degree, reducing process temperature, and thus decreasing energy consumption and limiting mechanical problems due to moderate conditions in a gasifier, as well as achieving a desired gas composition (Huang et al., 2015).
The coalbased integrated gasification combined cycle (IGCC) offers the advantages of higher efficiency in separating CO 2 and other pollutants compared to conventional coalfired power plants. The CO 2 collected in the IGCC can be injected into oceans or deep underground geological formations [4].
Electrochemical catalytic coal gasification experiments with Fuxin (FX) coal under a CO2 atmosphere were conducted to evaluate the effects of power and temperature on coal gasification and char structure evolution during electrochemical catalytic gasification (ECG). When the power was 400 W, with temperature increasing from 800 to 1000 °C, the CO content in the gas products increased by % ...
DOE PAGES ® Journal Article: Catalytic gasification of a Powder River Basin coal with CO2 and H2O mixtures. Catalytic gasification of a Powder River Basin coal with CO2 and H2O mixtures. Full Record; Other Related Research; Authors: Zhang, Fan; Fan, Maohong; Huang, Xin; Argyle, Morris D.; Zhang, Bo; Towler, Brian; Zhang, Yulong
Popa et al. [13]. studied the catalytic steam gasification of a Powder River Basin coal using Na 2 CO 3, and the results demonstrated that the total amounts of H 2, CO, CO 2 and CH 4 generated during the entire gasification with 5 g of dry ashfree coal were,, and mol, respectively, while correspondingly, those with catalyst ...
DOI: / Corpus ID: ; Catalytic gasification of a Powder River Basin coal article{Popa2013CatalyticGO, title={Catalytic gasification of a Powder River Basin coal}, author={T. Popa and Maohong Fan and Morris D. Argyle and Rachid B. Slimane and David A. Bell and Brian Towler}, journal={Fuel}, year={2013}, volume={103}, pages={161170}, url={https://api ...
The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO 2 and H 2 O mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the coal gasification.
CO2 capture and utilization caused more and more public attention because of its environmental impact. The objective of this work was to study the catalytic gasification of a subbituminous coal from the Powder River Basin (PRB) using a CO2 and H2O mixture as the gasifying agent. Sodium and iron, in the form of inexpensive compounds, were chosen to catalyze the ...
DOI: / Corpus ID: ; Characterization of the mechanism of gasification of a powder river basin coal with a composite catalyst for producing desired syngases and liquids
The objective of this research was to examine the mechanisms of FeCO 3, Na 2 CO 3, and FeCO 3Na 2 CO 3 based catalytic coal gasification of a lowsulfur subbituminous Wyodak coal from the Powder River Basin (PRB) of Wyoming. Xray diffraction (XRD), Mössbauer spectroscopy, scanning electron microscopy (SEM), Fourier transform infrared spectroscopy (FTIR), gas chromatography (GCMS) and ...
The catalytic effect of AAEMs on CSC gasification was weakened due to waterleaching treatment. ... Reaction kinetics of Powder River Basin coal gasification were measured in a modified drop tube ...
A study was carried out in both inert and CO 2 atmosphere to investigate the interaction mechanism of K 2 CO 3 with graphite and coal char during the catalytic gasification of coal char. The formation of K 2 CO 3 catalytic precursors was identified by using series of different techniques. The results obtained in an inert atmosphere show that the interaction between K 2 CO 3 and carbon readily ...
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Introduction. Nowadays, coal gasification technology is being widely developed to keep up with the soaring energy demand [1], [2]. Partial replacement of H 2 O by CO 2 to realize the gasification of coal with H 2 O/CO 2 mixtures (cogasification) is an important approach that can allow for green, lowcarbon, and sustainable development [3]. Moreover, low temperature gasification should also be ...
The mechanisms of char gasification in the mixture of H2O and CO2 are not clear, and some problems are yet to be solved. The LangmuirHinshelwood (LH) model of char gasification in the mixture of H2O and CO2 and the inhibition effect between charH2O and charCO2 reactions are two controversial issues among these problems. This paper presented new data to elucidate these two issues ...
In this study, DFT is used to search for possible CO2 gasification paths at the two char edges (armchair edge and zigzag edge) catalyzed by Fe. The optimal reaction path is determined by path ...
The catalytic gasification of coal using calcium as the catalyst has several advantages over potassium, such as lower costs and corrosiveness, abundant reserves on earth, and facile accessibility. ... 2015 Reaction kinetics of Powder River Basin coal gasification in carbon dioxide using a modified drop tube reactor. Fuel 140, 616625.
In this work, the influence of KCl concentration on the gasification characteristics of lignite coal char between °C is studied through the experiments of temperature programmed gasification and isothermal gasification using a thermogravimetric analyzer. The gasification kinetics, characteristic parameters, and the reaction mechanism of catalytic gasification is explored using the ...
Due to the serious impact of accelerating global climate change, the United States and China signed the China Joint Announcement on Climate Change in 2014, which imposed significant restrictions on the coal industry.
Variation of Char Reactivity during Catalytic Gasification with Steam: Comparison among Catalytic Gasification by IonExchangeable Na, Ca, and Na/Ca Mixture. ... Characterization of Powder River Basin coal pyrolysis with costeffective and environmentallyfriendly composite Na Fe catalysts in a thermogravimetric analyzer and a fixedbed reactor.
Abstract. Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na2CO3, widely available in ...
The YN coal samples were manually ground and sieved to particle sizes mm. The pyrolysis of coal samples and char gasification was carried out in a fixed bed reactor. The experimental setup is shown in Fig. 1. The quartz tube used in this work has an inner diameter of 5 cm and length of 22 cm, the
Popa et al. [13]. studied the catalytic steam gasification of a Powder River Basin coal using Na2CO3, and the results demonstrated that the total amounts of H2, CO, CO2 and CH4 generated during the entire gasification with 5 g of dry ashfree coal were,, and mol, respectively, while correspondingly, those with catalyst were ...
Catalytic gasification in the coal conversion process is a promising way to develop ... Wang, Y., Argyle, M. D. Fan, M. CO 2 gasification of powder river basin coal catalyzed by a costeffective ...
A kinetic characterization of the CO 2 gasification of chars from Chinese lowrank lignite coal is performed by isothermal thermogravimetry. The isothermal condition is 1,073 K, and the CO 2 concentration range is 1090%. Alkali and alkali earth catalysts were used to promote the gasification reactivity.
Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na 2 CO 3, widely available in Wyoming. Experiments were performed in an atmospheric pressure fixedbed laboratory gasifier.
Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na2CO3, widely available in Wyoming.
In the, Wyoming is well known for its abundance of coal, especially in the Powder River Basin region, which meets about 40% of coal demand. Thus people are highly interested in using Wyoming coal as a potential feedstock for producing liquid fuels.
CO 2 gasification of Wyodak lowsulfur subbituminous coal from the Powder River Basin (PRB) of Wyoming was conducted in a fixedbed laboratory gasifier at atmospheric pressure with Na 2 CO 3, an inexpensive catalyst widely available in sodium effect on the coal pyrolysis and the sodium forms existing during the char gasification were investigated using thermogravimetric analyses ...
The reason for this enhanced gasification is the fact that CaO, the main form of calcium mineral during coal catalytic gasification, ... Competition between H 2 O and CO 2 during the gasification of Powder River Basin coal. Fuel, Volume 187, 2017, pp. 94102. Ying Wang, David A. Bell.
Rapagnà et al. studied catalytic steam gasification of almond shells in a bubbling fluidizedbed gasifier by using 10 wt % of Fe/olivine catalyst synthesized via the impregnation method. (190) The experiments were performed at temperatures between 800 and 830 °C, and blank (olivine) was used for comparison of the effect of a catalyst on gas ...
Catalytic gasification of a Wyodak lowsulfur subbituminous coal from the Powder River Basin of Wyoming was investigated using an inexpensive catalyst, Na2CO3, widely available in Wyoming.
Steam gasification kinetics studies were conducted in a modified drop tube fixed bed reactor to approximate the injection of ambient temperature coal into a fluidized bed gasifier. Product gases were measured using a customized rapid response gas analysis system with a quadrupole mass spectrometer. Experiments were done within Regime I temperature range (no mass transfer restrictions), and ...
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